Journal
ADVANCED ENERGY MATERIALS
Volume 8, Issue 13, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/aenm.201702937
Keywords
carbon electrodes; hybrid devices; perovskites; photovoltaics; thermoelectric
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Funding
- National Natural Science Foundation of China [91733301, 91433203, 61474049, 21702069]
- Ministry of Science and Technology of China (863) [2015AA034601]
- 111 Project [B07038]
- Science and Technology Department of Hubei Province [2013BAA090]
- China Postdoctoral Science Foundation [2016M600588]
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An efficient perovskite photovoltaic-thermoelectric hybrid device is demonstrated by integrating the hole-conductor-free perovskite solar cell based on TiO2/ZrO2/carbon structure and the thermoelectric generator. The whole solar spectrum of AM 1.5 G is fully utilized with the approximate to 1.55 eV band gap perovskite (5-AVA)(x)(MA)(1-x)PbI3 absorbing the visible light and the carbon back contact absorbing the infrared light. The added thermoelectric generator improves the device performance by converting the thermal energy into electricity via the Seebeck effect. An optimized hybrid device is obtained with a maximum point power output of 20.3% and open-circuit voltage of 1.29 V under the irradiation of 100 mW cm(-2).
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