Searching for an exotic spin-dependent interaction with a single electron-spin quantum sensor

Searching for new particles beyond the standard model is crucial for understanding several fundamental conundrums in physics and astrophysics. Several hypothetical particles can mediate exotic spin-dependent interactions between ordinary fermions, which enable laboratory searches via the detection of the interactions. Most laboratory searches utilize a macroscopic source and detector, thus allowing the detection of interactions with submillimeter force range and above. It remains a challenge to detect the interactions at shorter force ranges. Here we propose and demonstrate that a near-surface nitrogen-vacancy center in diamond can be utilized as a quantum sensor to detect the monopole-dipole interaction between an electron spin and nucleons. Our result sets a constraint for the electron-nucleon coupling, g(s)(N)g(p)(e), with the force range 0.1-23 mu m. The obtained upper bound of the coupling at 20 mu m is g(s)(N)g(p)(e) < 6.24 x 10(-15).