Journal
WATER SCIENCE AND TECHNOLOGY
Volume 77, Issue 7, Pages 1931-1941Publisher
IWA PUBLISHING
DOI: 10.2166/wst.2018.073
Keywords
advanced treatment; biologically pretreated; catalytic ozonation; coal chemical industry wastewater; gas-liquid-solid internal circulating fluidized bed reactor
Funding
- National Natural Science Fund of China [51408158]
- China Postdoctoral Science Foundation [2017M612278]
- Natural Science Foundation of Shandong Province of China [ZR2017MEE020, ZR2017PEE008]
- Fundamental Research Funds for the Central Universities [HIT.NSRIF.2016098]
- scientific research foundation of Harbin institute of technology at Weihai [HIT(WH)201403]
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This paper investigated the performance of the combined system of catalytic ozonation and the gas-liquid-solid internal circulating fluidized bed reactor for the advanced treatment of biologically pretreated coal chemical industry wastewater (CCIW). The results indicated that with ozonation alone for 60 min, the removal efficiency of chemical oxygen demand (COD) could reach 34%. The introduction of activated carbon, pumice, gamma-Al2O3 carriers improved the removal performance of COD, and the removal efficiency was increased by 8.6%, 4.2%, 2%, respectively. Supported with Mn, the catalytic performance of activated carbon and gamma-Al2O3 were improved significantly with COD removal efficiencies of 46.5% and 41.3%, respectively; however, the promotion effect of pumice supported with Mn was insignificant. Activated carbon supported with Mn had the best catalytic performance. The catalytic ozonation combined system of MnOx/activated carbon could keep ozone concentration at a lower level in the liquid phase, and promote the transfer of ozone from the gas phase to the liquid phase to improve ozonation efficiency.
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