Journal
WATER RESOURCES
Volume 45, Issue 4, Pages 589-597Publisher
MAIK NAUKA/INTERPERIODICA/SPRINGER
DOI: 10.1134/S0097807818040139
Keywords
Fukushima; radiocesium; ponds; solution; particulate matter
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The article presents the results of studying radiocesium concentration and distribution between dissolved and particulate forms in ponds in the near zone of Fukushima Dai-ichi NPP NPP after the 2011 accident. The total concentration of Cs-137 in pond water and its variations are shown to be largely governed by the concentration of particulate matter being as high as 68 Bq/L, compared with 5 Bq/L in solution. The values of the distribution coefficient K-d in the ponds are similar to those in rivers and in large flow-through lakes in the accidentally polluted zone at Fukushima Dai-ichi NPP. The contributions of the main competing ions K+ and NH4+ to radiocesium desorption from solid particles into solution were similar for the ponds; however, their relative effect on dissolved radiocesium concentration varied over time because of variations in ammonium concentration.
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