Journal
TETRAHEDRON LETTERS
Volume 59, Issue 26, Pages 2600-2603Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tetlet.2018.05.069
Keywords
Peudolaric acids; Diterpenes; Dieckmann condensation; Trans-fused [5-7] ring system
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Funding
- Japan Society for the Promotion of Science [16K07712]
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Pseudolaric acids A (1) and B (2) are diterpene acids isolated from the root bark of Pseudolarix kaempferi as the main biologically active constituents of tujinpi, a traditional Chinese medicinal herb. Studies toward the total synthesis of 2 are described. The unusual trans-fused [5-7] ring system in the core structure of 2 was successfully synthesized via Dieckmann condensation. (C) 2018 Elsevier Ltd. All rights reserved.
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