4.8 Article

New 2D Carbon Nitride Organic Materials Synthesis with Huge-Application Prospects in CN Photocatalyst

Journal

SMALL
Volume 14, Issue 15, Pages -

Publisher

WILEY-V C H VERLAG GMBH
DOI: 10.1002/smll.201704138

Keywords

2D materials; CN photocatalysts; hydrogen evolution; layered; organic carbon nitride materials

Funding

  1. Taishan Scholar Program of Shandong Province
  2. Natural Science Foundation of Shandong Province [ZR2016JL015]
  3. National Natural Science Foundation of China [51572153, 51672109]
  4. Major Basic Program of the Natural Science Foundation of Shandong Province [ZR2017ZB0317]

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In recent years, 2D materials are attracting increased attention because of their excellent properties. In this paper, new 2D carbon nitride (CN) organic materials are successfully prepared on the basis of the organic synthesis theory, and the thickness is about 1.5 nm. This new 2D CN organic material further strengthens the 2D materials family. Meanwhile, their synthetic mechanism is theoretically speculated. Then CN photocatalysts of several structures are obtained by roasting 2D CN organic materials. Through the photocatalytic hydrogen production experiments, the results exhibit that these kinds of photocatalysts have good photocatalytic effects compared to common g-C3N4.

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