Journal
SMALL
Volume 14, Issue 11, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/smll.201703762
Keywords
CO2 reduction; lead-free; nanocrystals; perovskite; photochemistry
Categories
Funding
- National Natural Science Foundation of China [91433109]
- GDUPS
- Program of Guangzhou Science and Technology [201504010031]
- Fundamental Research Funds for the Central Universities
- NSF of Guangdong Province [S2013030013474]
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Lead halide perovskite nanocrystals (NCs) have demonstrated great potential as appealing candidates for advanced optoelectronic applications. However, the toxicity of lead and the intrinsic instability toward moisture hinder their mass production and commercialization. Herein, to solve such thorny problems, novel lead-free Cs2AgBiBr6 double perovskite NCs fabricated via a simple hot-injection method are reported, which exhibit impressive stability in moisture, light, and temperature. Such materials are then applied into photocatalytic CO2 reduction, achieving a total electron consumption of 105 mu mol g(-1) under AM 1.5G illumination for 6 h. This study offers a reliable avenue for Cs2AgBiBr6 perovskite nanocrystals preparation, which holds a great potential in the further photochemical applications.
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