Journal
SEPARATION AND PURIFICATION TECHNOLOGY
Volume 214, Issue -, Pages 11-20Publisher
ELSEVIER
DOI: 10.1016/j.seppur.2018.02.011
Keywords
Membrane distillation; Superhydrophobic membrane; Antifouling; Nucleation; Water treatment
Categories
Funding
- National Natural Science Foundation of China [21676043, 21527812, U1663223, 21606035]
- Changjiang Scholars Program [T2012049]
- Fundamental Research Funds for the Central Universities [DUT16TD19, DUT17213203]
- MOST innovation team in key area [2016RA4053]
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In this work, the superhydrophobic polypropylene (PP) composite membranes with modified surface were successfully fabricated by loading the SiO2 nanoparticles and attaching low surface energy 1H,1H,2H,2H-perfluorodecyltriethoxysilane. The impact of deposited nanoparticle size on the surface roughness, heterogeneous nucleation barrier and critical nucleus size versus the loaded nanoparticle size (d(nuclear)(*)/d) was simulated by the model combining the surface roughness and superhydrophobility with the critical nucleation energy. The optimized loaded nanoparticles size maintained the proper roughness and d(nuclear)(*)/d to ensure the desired performance of antifouling. The improved superhydrophobic surface enhanced the anti-wetting ability of the membrane for vacuum membrane distillation (VMD) purpose. The resulting modified membrane possessed good anti wetting ability and stable anti-fouling performance during long-term continuous and batch operation of VMD treating high salinity water system. The fouling rate of the fabricated membrane was decreased to 20% of the one of the original membrane under 15 wt% high salinity feed condition.
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