4.7 Article

Trans-boundary air pollution in a city under various atmospheric conditions

Journal

SCIENCE OF THE TOTAL ENVIRONMENT
Volume 618, Issue -, Pages 132-141

Publisher

ELSEVIER SCIENCE BV
DOI: 10.1016/j.scitotenv.2017.11.001

Keywords

Air pollution; Trans-boundary contribution; Non-negative matrix factorization; Tropical cyclones

Funding

  1. Chinese University of Hong Kong [2013/14, 4930059, 4930744]
  2. Early Career Scheme of Research Grants Council of Hong Kong [ECS-24301415]
  3. National Natural Science Foundation of China [41401052]

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Trans-boundary air pollution (TAP) is a crucial factor affecting air quality, and its contributionmay vary over time and differ under various atmospheric conditions. This study firstly applies an integrated statistical scheme to estimate the contributions of TAP and local sources to air pollutants in a city, and then investigate the influences of tropical cyclones (TC) on TAP. Hong Kong is chosen as an example because of its significant and special TAP characteristics. This study focuses on four major air pollutants, namely, respirable and fine suspended particulates (RSP/PM10 and FSP/PM2.5), sulfur dioxide (SO2), and nitrogen dioxide (NO2), from 2002 to 2013. Our results show that, on average, TAP is the major contributor of the annual RSP, FSP, SO2, and NO2 in Hong Kong. We estimate that when a TC is approaching, the increase in pollutant concentration in Hong Kong is mainly due to the increase in TAP contribution by the strengthened northerly wind at higher level of atmosphere (>= 900 hPa). These changes are accompanied by decreases in precipitation and increases in northerly/north-easterly wind, which may prolong the lifetime of pollutants, enhancing pollutant transport from mainland China to Hong Kong. (c) 2017 Elsevier B.V. All rights reserved.

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