Journal
PROGRESS IN NATURAL SCIENCE-MATERIALS INTERNATIONAL
Volume 28, Issue 2, Pages 121-132Publisher
ELSEVIER SCIENCE INC
DOI: 10.1016/j.pnsc.2018.02.001
Keywords
Heteroatom-doping; Functionalization, Carbon-based catalysts; Metal-free electrocatalysis, Energy conversion and storage
Funding
- NSF [CMMI-1400274]
- NSF (DOD-AFOSR-MURI) [FA9550-12-1-0037]
- NASA [NNX16AD48A, NNC16CA42C]
- National Natural Science Foundation of China [51732002]
- National Key Research and Development Program of China [2017YFA0206500]
- BUCT [buctylkxj02]
- National Basic Research Program of China [2011CB013000]
- Div Of Civil, Mechanical, & Manufact Inn
- Directorate For Engineering [1400274] Funding Source: National Science Foundation
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Recent development in nanoscience and nanotechnology has opened up new frontiers in materials science and engineering to create new materials for energy generation and storage. Owing to their earth abundance, low-cost, structural tunability, large-surface area, and unique physicochemical properties, graphitic carbon materials have attracted a great deal of attention for energy-related applications. However, the pristine graphene materials without functionalization is intractable (insoluble and infusible), which has hindered their practical applications. Therefore, considerable research effort has been devoted to the development of functionalized graphene materials with desirable properties for specific applications, including energy conversion and storage. It was demonstrated that functionalized graphene materials with tunable work functions were useful as charge-extraction materials to effectively improve solar cell performance while those with high electrocatalytic activities could be used as metal-free catalysts in fuel cells, metal-air batteries, water splitting and integrated energy systems. This article provides a timely focused review on the development of heteroatom-doped graphene materials for low-cost, but efficient, energy generation and storage.
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