4.8 Article

Energy dissipation and fluctuations in a driven liquid

Publisher

NATL ACAD SCIENCES
DOI: 10.1073/pnas.1713573115

Keywords

nonequilibrium thermodynamics; active matter; phase transitions

Funding

  1. University of Chicago
  2. UChicago Materials Research Science and Engineering Center - NSF [DMR-1420709]
  3. Sloan Fellowship

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Minimal models of active and driven particles have recently been used to elucidate many properties of nonequilibrium systems. However, the relation between energy consumption and changes in the structure and transport properties of these nonequilibrium materials remains to be explored. We explore this relation in a minimal model of a driven liquid that settles into a time periodic steady state. Using concepts from stochastic thermodynamics and liquid state theories, we show how the work performed on the system by various nonconservative, time-dependent forces-this quantifies a violation of time reversal symmetry-modifies the structural, transport, and phase transition properties of the driven liquid.

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