4.8 Article

Topological transformations of Hopf solitons in chiral ferromagnets and liquid crystals

Publisher

NATL ACAD SCIENCES
DOI: 10.1073/pnas.1716887115

Keywords

three-dimensional soliton; self-assembly; ferromagnetism; chirality

Funding

  1. US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [ER46921]
  2. National Science Foundation [ACI-1532235, ACI-1532236]

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Liquid crystals are widely known for their facile responses to external fields, which forms a basis of the modern information display technology. However, switching of molecular alignment field configurations typically involves topologically trivial structures, although singular line and point defects often appear as short-lived transient states. Here, we demonstrate electric and magnetic switching of nonsingular solitonic structures in chiral nematic and ferromagnetic liquid crystals. These topological soliton structures are characterized by Hopf indices, integers corresponding to the numbers of times that closed-loop-like spatial regions (dubbed preimages) of two different single orientations of rod-like molecules or magnetization are linked with each other. We show that both dielectric and ferromagnetic response of the studied material systems allow for stabilizing a host of topological solitons with different Hopf indices. The field transformations during such switching are continuous when Hopf indices remain unchanged, even when involving transformations of preimages, but discontinuous otherwise.

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