Journal
POLYMER CHEMISTRY
Volume 9, Issue 15, Pages 1938-1941Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8py00312b
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Funding
- U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES) [DE-SC0013906]
- American Academy of Arts and Sciences
- Alfred P. Sloan Foundation
- Johns Hopkins University
- U.S. Department of Energy (DOE) [DE-SC0013906] Funding Source: U.S. Department of Energy (DOE)
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Poly(cyclosilane)s, conjugated polymers inspired by crystalline silicon, are synthesized by group 4 metallocene-promoted dehydrocoupling polymerization. Changes in metallocene structure and reactivity are correlated with changes in poly(cyclosilane) chain length and optical properties. This work demonstrates the ability of target-directed synthesis to afford tunable, complex polymeric architectures.
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