Journal
ORGANIC LETTERS
Volume 20, Issue 15, Pages 4507-4511Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.8b01809
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Funding
- National Natural Science Foundation of China [21572154, 21772181, 21776148]
- NSFC-Shandong Joint Fund for Marine Science Research Centers [U1606403]
- Natural Science Foundation of Shandong Province [ZR2016BM07]
- Fundamental Research Funds for the Central Universities [201612013]
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A metal-free regio- and stereoselective method is achieved for the preparation of (E)-configured alpha-halo enamides, vinyl thioethers, and vinyl ethers using aqueous HX (X = F, Cl, Br, I), which features high functional group compatibility and regio- and stereoselectivity, mild conditions, high efficiency, and rapid transformation. Additionally, the isomers could be yielded readily from the (E)-configured a halo enamides via photocatalysis or under Sonogashira coupling conditions.
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