Journal
ORGANIC LETTERS
Volume 20, Issue 13, Pages 3975-3979Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.8b01540
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Funding
- Natural Science Foundation of Jiangsu Province [BK20171463]
- State Key Program of National Natural Science Foundation of China [21432009]
- Jiangsu students' project for innovation and entrepreneurship training program [201810291045Z]
- SICAM Scholarship by Jiangsu National Synergetic Innovation Center for Advanced Materials
- Nanyang Technological University
- SICAM Fellowship by Jiangsu National Synergetic Innovation Center for Advanced Materials
- Nanjing Tech University
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A regioselective formal [4 + 2] cycloaddition for the assembly of highly functionalized benzene rings was successfully developed. In this reaction, olefinic C-H bond functionalization/cyclization cascade reaction followed by rearomatization led to the desired molecules in one step under mild reaction conditions. This protocol also displays a broad substrate scope and good tolerance to a wide range of functional groups. Additionally, the potential utility for the synthesis of highly conjugated polybenzenes and diversification of natural products was also demonstrated.
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