Journal
ORGANIC LETTERS
Volume 20, Issue 7, Pages 1978-1981Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.8b00521
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Funding
- DFG [AN 1064/4-1]
- Boehringer Ingelheim Foundation
- Verband der Chemischen Industrie e.V.
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The nitrosonium ion-catalyzed dehydrogenative coupling of heteroarenes under mild reaction conditions is reported. The developed method utilizes ambient molecular oxygen as a terminal oxidant, and only water is produced as byproduct. Dehydrogenative coupling of heteroarenes translated into the rapid discovery of novel hedgehog signaling pathway inhibitors, emphasizing the importance of the developed methodology.
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