Journal
ORGANIC LETTERS
Volume 20, Issue 10, Pages 3074-3078Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.8b01114
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Funding
- National Natural Science Foundation of China [81403050, 81603000]
- NSFC-Joint Foundation of Yunnan Province [U1132604]
- Natural Science Foundation of Yunnan province [2016FB138]
- Yunnan Major Science and Technology Project [2015ZJ002]
- Foundation of State Key Laboratory of Phytochemistry and Plant Resources in West China [P2015-KF03]
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Pepluanols C and D (1 and 2), featuring unprecedented 5/5/10 with out,out-[7.2.1]bicylcododecane core and 6/6/7/3 fused-ring skeletons, respectively, were isolated from Euphorbia peplus. Their chemical structures and absolute configurations were determined by a series of extensive spectroscopic methods, and X-ray diffraction analysis. In addition, pepluanols C and D showed 31.6 +/- 8.3% and 30.5 +/- 2.8% peak current inhibition on the K(v)1.3 potassium channel at 30 mu M.
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