Journal
ORGANIC ELECTRONICS
Volume 59, Issue -, Pages 366-373Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.orgel.2018.05.050
Keywords
Non-fullerene polymer solar cells; Electron acceptors; Small molecules; Open-circuit voltage loss
Funding
- Ministry of Science and Technology [2014CB643501]
- Natural Science Foundation of China [91633301, 21490573, 51673069]
- Science and Technology Program of Guangzhou, China [201710010021, 201707020019, 2017A050503002]
- DFG [BR 4031/13-1, SFB 953]
- Bavarian Ministry of Economic Affairs and Media, Energy and Technology - HI-ERN of FZ Julich [IEK11]
- Aufbruch Bayern initiative of the state of Bavaria (EnCN)
- Bavarian Initiative Solar Technologies go Hybrid (SolTech)
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We report two novel small-molecule non-fullerene acceptors, IF-TN and IDT-TN, with indenofluorene (IF) and indacenodithiophene (IDT) as their respective central electron-rich cores and naphthyl-fused indanone (N) as the electron-withdrawing end-groups. By pairing these non-fullerene acceptors with a widely used polymer PBDB-T, the fabricated polymer solar cells based on PBDB-T: IDT-TN obtain a power conversion efficiency up to 5.89%, associated with a relatively high open-circuit voltage of 0.97 V and a remarkably low non-radiative open-circuit voltage loss of 0.23 V. These findings provide an effective approach for the rational molecular design of small-molecule acceptors with low non-radiative open-circuit voltage loss.
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