Journal
ORGANIC & BIOMOLECULAR CHEMISTRY
Volume 16, Issue 2, Pages 274-284Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7ob02670f
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Funding
- CSIR, New Delhi [01 (5234)/15]
- DST [YSS/2015/001552]
- CSIR
- RGNF
- IIESTS
- UGC
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A general, efficient and environmentally benign, one-step synthesis of substituted quinoline derivatives was achieved by acceptorless dehydrogenative coupling of o-aminobenzylalcohols with ketones and secondary alcohols catalyzed by a cheap, earth abundant and easy to prepare nickel catalyst [Ni(MeTAA)], featuring a tetraaza macrocyclic ligand (tetramethyltetraaza[14]annulene (MeTAA)). A wide variety of substituted quinolines were synthesized in high yields starting from readily available o-aminobenzylalcohols and ketones or secondary alcohols. A few controlled reactions were carried out to establish the acceptorless dehydrogenative nature of the reactions.
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