Journal
NEW JOURNAL OF CHEMISTRY
Volume 42, Issue 9, Pages 6750-6755Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8nj00940f
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Funding
- National Key Research and Development Program of China [2017YFA0205302]
- National Natural Science Foundation of China [61671250, 21475064, 21305070, 21605026, 81672720]
- Program for Changjiang Scholars and Innovative Research Team in University [IRT_15R37]
- Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD) [YX03002]
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Herein, a nonenzymatic electrochemical biosensor for glucose detection was developed based on an Au@Pt core-shell nanoparticle-decorated MoS2 (MoS2-Au@Pt) nanohybrid. Such designed MoS2-based nanohybrid possessed the advantages of MoS2 nanosheets with a large surface area and noble bimetallic nanoparticles with high catalytic ability, making the MoS2-Au@Pt nanocomposite modified electrode exhibit excellent electrocatalytic activity toward the oxidation of glucose due to their synergistic effect. As expected, the MoS2-based electrochemical biosensor showed a wide linear response over glucose concentration ranging from 10 mu M to 3 mM with a low detection limit of 1.08 mu M (S/N = 3). Furthermore, the as-prepared electrochemical biosensor also showed excellent selectivity and stability, which could be employed to determine glucose in real samples with acceptable results. The MoS2-Au@Pt nanohybrid could be a promising candidate material for the construction of a high performance sensing platform for chemical/biological molecule detection.
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