4.3 Article

Removal of Antibiotics From Water with an All-Carbon 3D Nanofiltration Membrane

Journal

NANOSCALE RESEARCH LETTERS
Volume 13, Issue -, Pages -

Publisher

SPRINGER
DOI: 10.1186/s11671-018-2555-9

Keywords

Antibiotics; Graphene oxide; Nanochannels; All-carbon membrane

Funding

  1. National Natural Science Foundation of China [21605062, 21375051, 21505057]
  2. Natural Science Foundation of Jiangsu Normal University [15XLR011]
  3. Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD)
  4. Brand Major of Universities in Jiangsu Province
  5. Top-notch Academic Programs Project of Jiangsu Higher Education Institution (TAPP)

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Recent industrial developments and increased energy demand have resulted in significantly increased levels of environmental pollutants, which have become a serious global problem. Herein, we propose a novel all-carbon nanofiltration (NF) membrane that consists of multi-walled carbon nanotubes (MWCNTs) interposed between graphene oxide (GO) nanosheets to form a three-dimensional (3D) structure. The as-prepared membrane has abundant two-dimensional (2D) nanochannels that can physically sieve antibiotic molecules through electrostatic interaction. As a result, the prepared membrane, with a thickness of 4.26 pm, shows both a high adsorption of 99.23% for tetracycline hydrochloride (TCH) and a high water permeation of 16.12 L m(-2) h(-1) bar(-1) In addition, the cationic dye methylene blue (MB) was also removed to an extent of 83.88%, indicating broad applications of the prepared membrane.

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