Journal
NANOSCALE
Volume 10, Issue 27, Pages 13270-13276Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8nr02932f
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Funding
- National Natural Science Foundation of China [NSFC - 21671170, 21673203, 21201010]
- Top-notch Academic Programs Project of Jiangsu Higher Education Institutions (TAPP)
- Program for New Century Excellent Talents of the University in China [NCET-13-0645]
- Innovation Scientists and Technicians Troop Construction Projects of Henan Province [164200510018]
- Six Talent Plan [2015-XCL-030]
- Qinglan Project
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Ultrathin two-dimensional (2D) metal-organic framework (MOF) nanosheets have been regarded as very promising electrocatalysts, although more efforts need to be devoted to improve their electrocatalytic activity. Here, we have developed ultrathin 2D nanosheet-assembled [Ni-3(OH)(2)(PTA)(2)(H2O)(4)]2H(2)O (Ni-MOF, PTA = p-benzenedicarboxylic acid) hierarchical flowers, which demonstrate superior electrocatalytic activity and excellent stability for the glucose oxidation reaction (GOR). The ultrathin 2D nanosheet-assembled flower-like nanostructure can provide interconnected open pores, accounting for its high electrocatalytic performance. Additionally, most of the ultrathin 2D nanosheets are in close contact with each other, making the ultrathin 2D nanosheets more stable. Furthermore, the electrocatalytic activity of the Ni-MOF flowers can be adjusted by doping Zn into the framework.
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