4.8 Article

Enhanced Single-Photon Emission from Carbon-Nanotube Dopant States Coupled to Silicon Microcavities

Journal

NANO LETTERS
Volume 18, Issue 6, Pages 3873-3878

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.8b01170

Keywords

Carbon nanotubes; photoluminescence; single-photon source; diazonium doping; photonic crystal

Funding

  1. JSPS (KAKENHI) [JP16K13613, JP17H07359]
  2. MEXT (Photon Frontier Network Program, Nanotechnology Platform)
  3. MERIT
  4. RIKEN Junior Research Associate Program
  5. Los Alamos National Laboratory Directed Research and Development funds

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Single-walled carbon nanotubes are a promising material as quantum light sources at room temperature and as nanoscale light sources for integrated photonic circuits on silicon. Here, we show that the integration of dopant states in carbon nanotubes and silicon microcavities can provide bright and high-purity single-photon emitters on a silicon photonics platform at room temperature. We perform photoluminescence spectroscopy and observe the enhancement of emission from the dopant states by a factor of similar to 50, and cavity-enhanced radiative decay is confirmed using time-resolved measurements, in which a similar to 30% decrease of emission lifetime is observed. The statistics of photons emitted from the cavity-coupled dopant states are investigated by photon-correlation measurements, and high-purity single photon generation is observed. The excitation power dependence of photon emission statistics shows that the degree of photon antibunching can be kept high even when the excitation power increases, while the single-photon emission rate can be increased to similar to 1.7 X 10(7) Hz.

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