Journal
NANO LETTERS
Volume 18, Issue 6, Pages 3716-3722Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.8b00861
Keywords
Perovskite; quantum dot; thermodynamic size control; ensemble uniformity
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Funding
- Robert A. Welch Foundation [A-1639]
- NSF [DMR-1404457]
- NSF GRFP [DGE-1252521]
- [IBS-R026-D1]
- Ministry of Science & ICT (MSIT), Republic of Korea [IBS-R026-D1-2018-A00] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
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Cesium lead halide (CsPbX3) nanocrystals have emerged as a new family of materials that can outperform the existing semiconductor nanocrystals due to their superb optical and charge-transport properties. However, the lack of a robust method for producing quantum dots with controlled size and high ensemble uniformity has been one of the major obstacles in exploring the useful properties of excitons in zero-dimensional nanostructures of CsPbX3. Here, we report a new synthesis approach that enables the precise control of the size based on the equilibrium rather than kinetics, producing CsPbX3 quantum dots nearly free of heterogeneous broadening in their exciton luminescence. The high level of size control and ensemble uniformity achieved here will open the door to harnessing the benefits of excitons in CsPbX3 quantum dots for photonic and energy-harvesting applications.
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