4.8 Article

Light-Emitting Halide Perovskite Nanoantennas

Journal

NANO LETTERS
Volume 18, Issue 2, Pages 1185-1190

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.7b04727

Keywords

Halide perovskites; photoluminescence; nanoantenna; Mie resonance; Purcell effect

Funding

  1. Ministry of Education and Science of the Russian Federation [14.Y26.31.0010]
  2. Russian Science Foundation [17-73-20336]
  3. Australian Research Council
  4. Welch Foundation [AT 16-17]
  5. Russian Science Foundation [17-73-20336] Funding Source: Russian Science Foundation

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Nanoantennas made of high-index dielectrics with low losses in visible and infrared frequency ranges have emerged as a novel platform for advanced nanophotonic devices. On the other hand, halide perovskites are known to possess high refractive index, and they support excitons at room temperature with high binding energies and quantum yield of luminescence that makes them very attractive for all-dielectric resonant nanophotonics. Here we employ halide perovskites to create light-emitting nanoantennas with enhanced photoluminescence due to the coupling of their excitons to dipolar and multipolar Mie resonances. We demonstrate that the halide perovskite nanoantennas can emit light in the range of 530-770 nm depending on their composition. We employ a simple technique based on laser ablation of thin films prepared by wet-chemistry methods as a novel cost-effective approach for the fabrication of resonant perovskite nanostructures.

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