Journal
MATERIALS RESEARCH BULLETIN
Volume 100, Issue -, Pages 56-61Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.materresbull.2017.12.003
Keywords
Ca14Al10Zn6O35; Phosphors; Energy transfer; Bi3+Sm3+
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Funding
- National Natural Science Foundation of China [21371062, 21671070, 21571067]
- Project for Construction of High-level University in Guangdong Province
- Guangdong Natural Science Foundation [S2013030012842]
- Provincial Science and technology project of Guangdong Province [2016A050502043]
- Guangzhou Science & Technology Project [201704030086, 201605030005]
- Spectral Funds for the Cultivation of Guangdong College Student Scientific and Technological Innovation (Climbing Program Special Funds) [pdjh2017a0075]
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A series of Bi3+ Sm3+-codoped Ca14Al10Zn6O35 phosphors were synthesized via conventional high temperature solid-state method. The crystal structure, morphology, photoluminescence and energy transfer mechanism from Bi3+ to Sm3+ were investigated in detail. A broad blue emission band due to P-3(1) -> S-1(0) transition of Be3+ was observed in the Bi3+ single-doped Ca14Al10Zn6O35 sample, the Ca2+ position are verified to be replaced by Bi3+ and the corresponding concentration quenching mechanism was dipole-dipole interaction. The considerable spectral overlap between the broad emission band of Bi3+ around 350-550 nm and the excitation band of Sm3+ supports the energy transfer from Bi3+ to Sm3+. This investigation will contribute to the comprehension of interactions between Bi3+ and Sm3+. These results reveal the potential application of Bi3+, Sm3+ co-doped phosphor in UV light-emitting diodes and artificial light in plant.
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