Journal
MATERIALS LETTERS
Volume 214, Issue -, Pages 290-292Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.matlet.2017.12.017
Keywords
Rhodium catalysts; Autothermal reforming; N-hexadecane; Diesel; Nanoparticles; Interfaces
Funding
- Ministry of Education and Science of Russian Federation [14.607.21.0149, RFMEFI60716X0149]
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Highly dispersed Rh particles supported on Ce0.75Zr0.25O2-delta mixed with alumina were prepared by sorption-hydrolytic deposition technique. Produced catalyst exhibited high activity in autothermal reforming of n-hexadecane, but suffered from coking. Structured Rh/Ce0.75Zr0.25O2-delta-eta-Al2O3/FeCrAl catalyst was prepared by strongly bound catalytic coating deposition onto metallic wire mesh to provide effective heat transfer and avoid coking. Rh/Ce0.75Zr0.25O2-delta-eta-Al2O3/FeCrAl showed excellent performance in n-hexadecane autothermal reforming providing 100% conversion and stable operation for at least 12 h on stream without detection of any carbon deposits. (C) 2017 Elsevier B.V. All rights reserved.
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