4.6 Article

Facile synthesis of carbon-doped g-C3N4 for enhanced photocatalytic hydrogen evolution under visible light

Journal

MATERIALS LETTERS
Volume 212, Issue -, Pages 111-113

Publisher

ELSEVIER SCIENCE BV
DOI: 10.1016/j.matlet.2017.10.079

Keywords

Carbon materials; Semiconductors; g-C3N4; Doping; Photocatalysis; Hydrogen production

Funding

  1. National Nature Science Foundation of China [21606111, 21406091]
  2. Natural Science Foundation of Jiangsu Province [BK20140530, BK20150482]
  3. China Postdoctoral Science Foundation [2015M570409]
  4. Research Foundation for Talented Scholars of Jiangsu University [15JDG054]

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We demonstrated a facile synthesis of carbon-doped g-C3N4 (donated as C-CN) photocatalyst for hydrogen evolution. The obtained C-CN photocatalyst showed a H-2 production rate of 40.37 mu molh 1 under visible light irradiation (lambda > 420 nm), which is about 2.9 times of that over bare CN. The enhanced photocatalytic activity of C-CN can be ascribed to enhanced visible light adsorption and improved charge carrier separation, which is probably resulted from the delocalized TC bonds generated after C doping. It is anticipated that our work could provide a feasible way to improve the photocatalytic performance of CN. (C) 2017 Elsevier By. All rights reserved.

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