Journal
MACROMOLECULES
Volume 51, Issue 14, Pages 5346-5351Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.macromol.8b01224
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Funding
- EPSRC [EP/L017393/1, EP/K014668/1]
- EIT Climate KIC (project EnCO2re)
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Well-defined pentablock copolymers are prepared using a single catalyst, in one pot, from four different monomers: anhydride, epoxide, lactone, and CO,. The dizinc catalyst bridges three distinct polymerization cycles and performs a double switch in polymerization mechanism to produce pentablock copolymers. The new materials are hydroxyl-telechelic and are efficiently postfunctionalized to introduce polar and nonpolar side-chains.
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