Journal
JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A
Volume 36, Issue 3, Pages -Publisher
A V S AMER INST PHYSICS
DOI: 10.1116/1.5021587
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Funding
- U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]
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Application of the linear least squares (LLS) methodology allows for quantitative determination of variation in material composition with depth. LLS fits were applied to decompose and enhance the interpretation of spectra obtained by Auger electron spectroscopy during depth profiles of oxidized plutonium surfaces. By means of the LLS algorithm, chemical state assignments of the Pu P1VV/O45VV, O KLL, and C KLL Auger transitions were determined and the existence of a subsurface oxycarbide layer was identified, with confirmation of the oxide and metal components provided from comparison to previous measurements of standard samples. Published by the AVS.
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