Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 140, Issue 31, Pages 9788-9792Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.8b03718
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Funding
- JSPS KAKENHI [17K19126, 16H04150, 15H0S839, 16H01040, 18H04271]
- Research Grant of Keio Leading-edge Laboratory of Science Technology
- Grants-in-Aid for Scientific Research [16H01040, 17K19126, 18H04271, 16H04150] Funding Source: KAKEN
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A novel method for direct transformation of allyl groups in allylbenzene derivatives to alkenyl groups via rhodium-catalyzed C-C bond cleavage is reported. The alkenylation with styrenes of allylbenzenes containing pyridyl and pyrazolyl groups as a directing group proceeded efficiently to give alkenylation products. We also developed a new protocol for transformation of an ortho-prenylated phenol to an aniline derivative.
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