Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 140, Issue 21, Pages 6545-6549Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.8b03509
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Funding
- Scripps Research Institute
- NIH [NIGMS 2R01 GM084019]
- Shanghai RAAS Blood Products Co. Ltd.
- NATIONAL INSTITUTE OF GENERAL MEDICAL SCIENCES [R01GM084019] Funding Source: NIH RePORTER
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A monoprotected aminoethyl amine chiral ligand based on an ethylenediamine backbone was developed to achieve Pd-catalyzed enantioselective C(sp(3))-H arylation of cyclopropanecarboxylic and 2-aminoisobutyric acids without using exogenous directing groups. This new chiral catalyst affords new disconnection for preparing diverse chiral carboxylic acids from simple starting materials that are complementary to the various ring forming approaches.
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