Journal
JOURNAL OF POWER SOURCES
Volume 396, Issue -, Pages 566-573Publisher
ELSEVIER
DOI: 10.1016/j.jpowsour.2018.06.044
Keywords
Graphene nanoribbons; Dye sensitized solar cells; TiO2-GNR hybrid photoanodes; Electron transport; Carrier recombination
Funding
- Natural Science and Engineering Research Council of Canada (NSERC)
- Canada Foundation for Innovation
- government of China
- Sichuan province
- IFFS/UESTC
- Postdoctoral Science Foundation of China
- Canada Research Chairs program
- INTERNEW EU project (FEDER) [MAT2017-82970-C2-2-R]
- Aragon regional government (Construyendo Europa desde Aragon) [E13_17R, E28_17R]
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We report the effect of incorporating different loadings of graphene nanoribbons (GNR) into a standard photoanode made of TiO2 sensitized with dye molecules. The GNRs are observed to significantly improve the photoconversion efficiency (PCE) of dye-sensitized solar cells (DSSCs). The TiO2-GNR hybrid photoanodes were prepared using the doctor-blade method. The presence of GNR in the composite photoanode was characterized by scanning electron microscopy, transmission electron microscopy and Raman spectroscopy. Our results highlight that, at an optimum loading of 0.005 wt%, GNR increases the PCE of DSSCs up to values 20% higher than the PCE of control devices. This improvement is mainly attributed to improved dye loading, enhanced electron lifetime and reduced carrier recombination, as confirmed by quantitative measurements of dye loading, transient photovoltage decay and electrochemical impedance spectroscopy results, respectively.
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