Journal
JOURNAL OF PHYSICAL CHEMISTRY C
Volume 122, Issue 14, Pages 7621-7626Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.jpcc.8b01264
Keywords
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Funding
- European Research Council (ERC) under the European Union's Horizon research and innovation programme [725165]
- Spanish Ministry of Economy and Competitiveness (MINECO)
- Fondo Europeo de Desarrollo Regional (FEDER) [MAT2014-56210-R]
- MINECO under the program Redes de Excellencia TFE
- Fundacio Privada Cellex
- program CERCA
- Spanish Ministry of Economy and Competitiveness, through the Severo Ochoa Programme for Centres of Excellence in RD [SEV-20150522]
- two Marie Curie Standard European Fellowships [H2020-MSCA-IF-2015-703018, H2020-MSCA-IF-2016-750600]
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Lead halide perovskite nanocrystals (NCs) are currently emerging as one of the most interesting solution-processed semiconductors because they possess high photoluminescence quantum yield (PLQY) and color tunability through anion exchange reactions or quantum confinement. Here, we show efficient solar cells based on mixed-halide (CsPbBrI2) NCs obtained via anion exchange reactions under ambient conditions. We performed anion exchange reactions in concentrated NC solutions with I-, thus inducing a PL red shift up to 676 nm and obtaining a high PLQY in film (65%). Solar cell devices operating in the wavelength range 350-660 nm were fabricated in air with two different deposition methods. The solar cells display a photoconversion efficiency of 5.3% and open circuit voltage (V-oc) up to 1.31 V, among the highest reported for perovskite-based solar cells with band gap below 2 eV, clearly demonstrating the potential of this material.
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