Journal
GREEN CHEMISTRY
Volume 17, Issue 2, Pages 1107-1112Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4gc01814a
Keywords
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Funding
- MOST [2011CBA00504]
- NSFC of China [21133010, 51221264, 21261160487]
- Chinese Academy of Sciences [XDA09030103]
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A new concept of ionic liquid (IL) mono-dispersing catalyst on nanocarbon surface is presented. The liquid mixture of IL and model catalyst (1-octyl-3-methyl imidazolium phosphotungstate, OPW) on carbon nanotube is in a solid state which can be easily characterized and give a fundamental understanding of the interaction between the catalyst and the IL. The condensed IL is found to weaken the W=O bond of a catalyst that favours its interaction with an oxidizing agent that exhibited a reaction rate of 176 times to the performance of a single OPW during the oxidation of dibenzothiophene. Due to the hetero-genization of this system, the catalyst can be easily recycled by a simple gravity separation.
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