4.4 Article Proceedings Paper

Radiocaesium derived from the TEPCO Fukushima accident in the North Pacific Ocean: Surface transport processes until 2017

Journal

JOURNAL OF ENVIRONMENTAL RADIOACTIVITY
Volume 189, Issue -, Pages 93-102

Publisher

ELSEVIER SCI LTD
DOI: 10.1016/j.jenvrad.2018.03.014

Keywords

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Funding

  1. Ministry of Education, Culture, Sports, Science and Technology Japan (KAKENHI) [24110005]
  2. EC [604974]
  3. Institute of Environmental Radioactivity, Fukushima University, Japan
  4. Joint Japan Ukraine project [SFFR 868/12879]
  5. Japan Society for the Promotion of Science
  6. State Fund for Fundamental Research under the Japan - Ukraine Research Cooperative Program [16932059]
  7. University of Tsukuba
  8. Hirosaki University [HF-7]
  9. Grants-in-Aid for Scientific Research [17K05652, 15K00520] Funding Source: KAKEN

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We report temporal variations of Cs-137 activity concentrations in surface waters of six regions of the western and central North Pacific Ocean during 2011-2017 using a combination of 1264 previously published data and 42 new data. In the western and central North Pacific Ocean at latitudes of 30-42 degrees N and longitudes of 140 degrees E to 160 degrees W, eastward transport of radiocaesium was clearly apparent. Cs-137 activity concentrations in surface water decreased rapidly to similar to 2-3 Bq m(-3) in 2015/2016, still a bit higher than Cs-137 activity concentrations before the FNPP1 accident (1.5-2 Bq m(-3)). Cs-134/Cs-137 activity ratios decay-corrected to 11 March 2011 were similar to 0.5-0.8. To the south of 30 degrees N and between 130 degrees E and 160 degrees W in the western and central Pacific Ocean, Cs-137 activity concentrations were around 1-7 Bq m(-3) in 2011/2012 but then stabilized at a few Bq m(-3) up to 2017.Cs-134 activity concentrations were detected at levels of 0.1-0.9 Bq m(-3), and Cs-134/Cs-137 activity ratios decay-corrected to 11 March 2011 were similar to 0.3-0.5. Temporal variations of model-simulated Cs-137 activity concentrations in surface water in the region of interest showed good agreement with observations, except in the southwestern North Pacific Ocean.

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