Journal
ACS APPLIED MATERIALS & INTERFACES
Volume 7, Issue 2, Pages 1031-1034Publisher
AMER CHEMICAL SOC
DOI: 10.1021/am5068436
Keywords
monodisperse; Ni; Pt; hydrazine; hydrogen storage
Funding
- National Natural Science Foundation of China [21201134]
- Natural Science Foundation of Jiangsu Province [BK20130370]
- Natural Science Foundation of Hubei Province [2013CFB288]
- Creative Research Groups of Hubei Province [2014CFA007]
- Large-scale Instrument and Equipment Sharing Foundation of Wuhan University
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Ultrafine monodisperse bimetallic NiPt nanoparticles with different compositions have been successfully synthesized by coreduction of nickel acetylacetonate and platinum acetylacetonate with borane-tert-butylamine in oleylamine. Among all the catalysts tested, Ni84Pt16/graphene exhibited 100% hydrogen selectivity, and marked high catalytic activity, with TOF values of 415 h(1) at 50 degrees C, and 133 h(1) at 25 degrees C for hydrogen generation from alkaline solution of hydrazine.
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