Journal
JOURNAL OF CHEMICAL PHYSICS
Volume 148, Issue 10, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.5023645
Keywords
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Funding
- Deutsche Forschungsgemeinschaft (DFG) through the excellence cluster The Hamburg Center for Ultrafast Imaging-Structure, Dynamics and Control of Matter at the Atomic Scale (CUI) [EXC1074]
- Deutsche Forschungsgemeinschaft (DFG) through the priority program Quantum Dynamics in Tailored Intense Fields (QUTIF) [1840, KU1527/3]
- European Research Council through the Consolidator Grant COMOTION [ERC-Kupper-614507]
- Helmholtz Association Initiative and Networking Fund
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Strong quasi-adiabatic laser alignment of the indole-water-dimer clusters, an amino-acid chromophore bound to a single water molecule through a hydrogen bond, was experimentally realized. The alignment was visualized through ion and electron imaging following strong-field ionization. Molecular-frame photoelectron angular distributions showed a clear suppression of the electron yield in the plane of the ionizing laser's polarization, which was analyzed as strong alignment of the molecular cluster with < cos(2) theta(2D)> >= 0.9. Published by AIP Publishing.
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