Journal
JOURNAL OF CHEMICAL PHYSICS
Volume 148, Issue 21, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.5032295
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Funding
- Deutsche Forschungsgemeinschaft (DFG) [Sonderforschungsbereich SFB-1319]
- Lichtenberg-Hochleistungsrechner of the Technische Universitat Darmstadt [0628, 0660]
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Angle-resolved multiphoton ionization of fenchone and camphor by short intense laser pulses is computed by the time-dependent single center method. Thereby, the photoelectron circular dichroism (PECD) in the three-photon resonance enhanced ionization and four-photon above-threshold ionization of these molecules is investigated in detail. The computational results are in satisfactory agreement with the available experimental data, measured for randomly oriented fenchone and camphor molecules at different wavelengths of the exciting pulses. We predict a significant enhancement of the multiphoton PECD for uniaxially oriented fenchone and camphor. Published by AIP Publishing.
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