Journal
JOURNAL OF ALLOYS AND COMPOUNDS
Volume 749, Issue -, Pages 811-817Publisher
ELSEVIER SCIENCE SA
DOI: 10.1016/j.jallcom.2018.03.378
Keywords
Prussian blue; Graphene foam; Composite; Anode; Lithium-ion batteries
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Funding
- National Natural Science Foundation [51672114]
- Natural Science Foundation of Jiangsu Province [BK20151328, BK20161357]
- Foundation from Marine Equipment and Technology Institute for Jiangsu University of Science and Technology [HZ20170015]
- Priority Academic Program Development of Jiangsu Higher Education Institutions
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The integration of active materials into graphene foam (GF) is of fundamental importance for developing superior binder-free electrodes. In the present design, Prussian blue (PB) nanocubes were uniformly grown into the GF network by a facile immersion approach. This is the first example of GF supported metal cyanides and their applications as electrode materials. The as-prepared PB and GF/PB samples have been characterized systematically. This free-standing and flexible GF/PB composite electrode exhibited a high reversible gravimetric (areal) capacity of 514mAh g(-1) (0.47 mAh cm(-2)) at 100 mA g(-1) over 150 cycles and superior cycling stability with 99% capacity retention as well as good rate capability of similar to 150 mAh g(-1) at 1 A g(-1). Such outstanding electrochemical behaviors were attributed to the synergistic integration of both GF and PB components. Thus, the GF/PB system can be employed as potential superior binder-free anode candidates for high-performance lithium-ion batteries. (C) 2018 Elsevier B.V. All rights reserved.
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