Journal
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
Volume 57, Issue 10, Pages 3602-3609Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.iecr.7b05301
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Funding
- Austrian Science Fund (FWF) [P 27410-N28]
- Austrian Research Promotion Agency (FFG) [FFGP13760002]
- European Union
- EFRE [RU2-EU-124/100-2010]
- ETC Austria-Czech Republic [M00146]
- Austrian Science Fund (FWF) [P27410] Funding Source: Austrian Science Fund (FWF)
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Herein, we present the design, synthesis, and characterization of fully degradable, hybrid, star-branched dendritic polyols. First multiarmed polyphosphazenes were prepared as a star branched scaffold which upon functionalization produced globular branched hydroxyl-functionalized polymers with over 1700 peripheral functional end groups. These polyols with unique branched architectures could be prepared with controlled molecular weights and relatively narrow dispersities. Furthermore, the polymers are shown to undergo hydrolytic degradation to low molecular weight degradation products, the rate of which could be controlled through postpolymerization functionalization of the phosphazene backbone.
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