Journal
ENERGY & ENVIRONMENTAL SCIENCE
Volume 11, Issue 4, Pages 988-994Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8ee00019k
Keywords
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Funding
- Danish Innovation Fund (4 M center)
- Danish DFF [4184-00332]
- Villum Foundation V-SUSTAIN [9455]
- Toyota Central RD Lab., Inc.
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In this work, we introduce the application of gas diffusion electrodes (GDE) for benchmarking the electrocatalytic performance of high surface area fuel cell catalysts. It is demonstrated that GDEs offer several inherent advantages over the state-of-the-art technique, i.e. thin film rotating disk electrode (TF-RDE) measurements for fast fuel cell catalyst evaluation. The most critical advantage is reactant mass transport. While in RDE measurements the reactant mass transport is severely limited by the gas solubility of the reactant in the electrolyte, GDEs enable reactant transport rates similar to technical fuel cell devices. Hence, in contrast to TF-RDE measurements, performance data obtained from GDE measurements can be directly compared to membrane electrode assembly (MEA) tests. Therefore, the application of GDEs for the testing of fuel cell catalysts closes the gap between catalyst research in academia and real applications.
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