Journal
ELECTROCHIMICA ACTA
Volume 270, Issue -, Pages 490-500Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.electacta.2018.03.090
Keywords
All-in-one supercapacitor; Polypyrrole; Graphene oxide; Electroless plating
Categories
Funding
- National Natural Science Foundation of China [21574076, U1510121, 21501113, 61504076, 21407100]
- National Natural Science Foundation of Shanxi province [2015021129]
- Program for the Top Young and Scientific and Technological Innovation Programs of Higher Education Institutions in Shanxi [020352901014]
- Fund for Shanxi 1331 Project Collaborative Innovation Center
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Sandwich-structured composite films with two conductive surface separated by porous insulator have been fabricated after the two sides of porous polypropylene films (PPF) have been covered with gold films via electroless plating method. Subsequently, the composite of polypyrrole-graphene oxide (PPyGO) has been electrochemically deposited on the two conductive sides via galvanostatic method to form the sandwich structured PPy-GO/PPF/PPy-GO composite films. After gel electrolyte of H3PO4/polyvinyl alcohol being coated on the composite films of PPy-GO/PPF/PPy-GO, the integrated flexible supercapacitors (SCs) of PPy-GO//PPF//PPy-GO are fabricated, and the optimal SCs exhibits excellent cycling stability (84.9% capacitance retention after 10000 cycles). Based on the one side electrode, the optimal SCs exhibit relatively high areal specific capacitance (108.0 mF cm(-2) at 2 mV s(-1) scanning rate). The integrated SCs exhibit excellent flexibility, the capacitance retention can reach 93.4% after 2000 bending cycles and 80.0% after 5000 bending cycles. Furthermore, this kind of integrated flexible capacitors can be conveniently connected in series without further wires due to their special structure. As a result, they display great potential in flexible and solid integrated energy storage systems. (C) 2018 Elsevier Ltd. All rights reserved.
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