Journal
DYES AND PIGMENTS
Volume 151, Issue -, Pages 7-14Publisher
ELSEVIER SCI LTD
DOI: 10.1016/j.dyepig.2017.12.037
Keywords
DSSC; Electrocatalytic; MoS2; CBD
Funding
- Ministry of Trade, Industry and Energy (MOTIE) [10051565]
- Korea Display Research Corporation (KDRC)
- GRRC program of Gyeonggi province [GRRC AJOU 2016803]
- Ministry of Trade, Industry and Energy under Sensor Industrial Technology Innovation Program [10063682]
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Interests in the development of economical and high-efficiency counter electrodes (CEs) of dye-sensitized solar cell (DSSC) to replace the excessively cost and scarce platinum (Pt) CEs have been increased. In this report, we demonstrate a facile chemical bath deposition (CBD) route to prepare layered MoS2/fluorine-doped tin oxide (FTO) films that directly act as the CEs of DSSCs. A DSSC containing the CBD-synthesized MoS2/FTO CE (prepared at 0.03 M Mo source concentration, 90 degrees C bath temperature and 30 min deposition time) exhibits high power conversion efficiency (PCE) of 7.14%, which is approaching that of DSSC with Pt/FTO CE (8.73%). The electrocatalytic activity of the MoS2/FTO and Pt/FTO CEs are discussed in detail with their cyclic voltammetry (CV), Tafel polarization curves, and electrochemical impedance spectra (EIS). The observed results indicate that our low-cost CE has a high electrocatalytic activity for the reduction of triiodide to iodide and a low charge transfer resistance at the electrolyte-electrode interface with a comparable state to that of a Pt/FTO CE.
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