Journal
DALTON TRANSACTIONS
Volume 47, Issue 6, Pages 1772-1776Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7dt04813k
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Funding
- Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences Heavy Element Chemistry Program of the U.S. Department of Energy (DOE) at LBNL [DE-AC02-05CH11231]
- Department of Energy National Nuclear Security Administration (Nuclear Science and Security Consortium) [DE-NA0003180, DE-NA0000979]
- German Academic Exchange Service (DAAD)
- NIH [S10-RR027172]
- Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]
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The syntheses of the first homoleptic U(III) and U(IV) amidate complexes are described. These can be interconverted by chemical reduction/oxidation, showing an unusual change in coordination number from four in the U(III) complex to eight in the U(IV) complex in the solid state structures.
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