Journal
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
Volume 548, Issue -, Pages 10-18Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.colsurfa.2018.03.039
Keywords
beta-Cyclodextrin; Copolymer; Silica nanoparticles; Rheology
Categories
Funding
- National Natural Science Foundation of China [51674270]
- National Major project [2017ZX05009-003]
- Major project of the National Natural Science Foundation of China [51490650]
- Foundation for Innovative Research Groups of the National Natural Science Foundation of China [51521063]
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Maleic anhydride modified beta-cyclodextrin (MAH-beta-CD) was copolymerized with acrylamide (AM) and 2-acry-lamido-2-methyl propane sulfonic acid (AMPS) to form a copolymer (denoted as AAMC) through redox free-radical polymerization. The copolymer was characterized by FT-IR, H-1 NMR and thermal gravimetric analysis. The silica nanoparticles suspension was mixed with AAMC solution, and their rheological properties were investigated under different experimental conditions. Results showed that AAMC/silica hybrid exhibited viscosity enhancement and better salt-resistance, temperature-tolerance and shear-resistance than AAMC. The AAMC/silica hybrid showed an impressive thermal stability at T = 85 degrees C after 15 days, and the viscosity reached about 2.5 times that of AAMC at 0.8 wt% nanoparticle loading. Dynamic rheology studies indicated that silica nanoparticles acted as physical crosslinkers among polymer molecules so as to enhance the elasticity of the AAMC/silica hybrid. The superior properties of AAMC/silica hybrid indicated that it has the potential to enhanced oil recovery.
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