Journal
CHINESE JOURNAL OF CHEMISTRY
Volume 36, Issue 7, Pages 644-659Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cjoc.201700742
Keywords
carbon dioxide; carboxylative cyclization; electrochemistry; photocatalysis; sustainable chemistry
Categories
Funding
- National Natural Science Foundation of China [21472103, 21672119, 21421001]
- National Key Research and Development Program [2016YFA0602900]
- Natural Science Foundation of Tianjin [16JCZDJC39900]
- 12th Five-Year National Science and Technology Support Plan [2015BAD15B07]
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In the last few years, photochemical and electrochemical CO2 transformations have attracted increasing attention in response to topical interest in renewable energy and green chemistry. The present minireview offers an overview about the current approaches for the photochemical and electrochemical carbon dioxide fixation with organic compounds. Valuable products, including carboxylic acids and heterocyclic compounds, are accessible through carboxylation and carboxylative cyclization, respectively. In photochemical and electrochemical processes, photo- or electro-induced radical ions or other high-energy organic compounds are considered as key intermediates to react with CO2. Besides, activation of CO2 to produce radical anion has also been reported.
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