Journal
CHEMISTRY-AN ASIAN JOURNAL
Volume 13, Issue 4, Pages 390-394Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/asia.201800020
Keywords
cucurbit[8]urils; fluorescence; host-guest systems; hydrogen evolution; supramolecular organic frameworks
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Funding
- Creative Research Initiative Program through the National Research Foundation of Korea (NRF) - Ministry of Science, ICT & Future Planning (MSIP) [2009-0081571[RIAM0417-20150013]]
- Global Frontier R&D Program on Center for Multiscale Energy System through the NRF - MSIP [2012M3A6A7055540]
- Basic Science Research Program through the NRF - Ministry of Science, ICT and Future Planning [2017R1E1A1A01075372]
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A highly fluorescent (phi(F)=0.60) and water-soluble two-dimensional (2D) honeycomb-shaped supramolecular organic framework (SOF) was successfully synthesized in pure aqueous solution via self-assembly of novel cyanostilbene-functionalized trilateral guest molecules and cucurbit[8]uril hosts. The size of this fluorescent 2D SOF was >500nm in diameter, 1.7nm in thickness, and 3.9nm in the honeycomb pore diameter. This 2D SOF holds potential as a new all-organic photosensitizer template for photocatalytic H-2 evolution from pure water.
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