Journal
CHEMICAL COMMUNICATIONS
Volume 54, Issue 63, Pages 8745-8748Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8cc04526g
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Funding
- National Natural Science Foundation of China [21625203, 21472039]
- Jiangxi Province Science and Technology Project [20165BCB18007, 20171ACB20015]
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A mild and general visible light photoredox catalysis-induced intermolecular three-component alkene 1,2-diarylation involving aryl C(sp(2))-H functionalization is described. The key to controlling the chemoselectivity toward alkene 1,2-diarylation is the employment of a 2,2'-bipyridine base, thus allowing the formation of two new C(sp(3))-C(sp(2)) bonds via aryl radical formation from aryldiazonium salts, addition across the C=C bonds, and aryl C(sp(2))-H functionalization cascades.
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