Journal
CHEMICAL COMMUNICATIONS
Volume 54, Issue 56, Pages 7770-7773Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8cc02300j
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Funding
- Swedish Research Council
- Swedish Energy Agency
- Knut & Alice Wallenberg Foundation
- European Research Council [ERC-CoG2015-681895_MOFcat]
- DST-INSPIRE [DST/INSPIRE/04/2017/001072]
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The molecular water oxidation catalyst [Ru(bda)(L)(2)] has been incorporated into pyridine-decorated MIL-101(Cr) metal-organic frameworks. The resulting MIL-101@Ru materials exhibit turnover frequencies (TOFs) up to ten times higher compared to the homogenous reference. An unusual dependence of the formal TOFs on oxidant concentration is observed that ultimately arises from differing amounts of catalysts in the MOF crystals being active.
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